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Enhanced Sensitivity in the Detection of 129I Using Accelerator Mass Spectrometry at the University of Notre Dame

PSB-66
23 Oct 2024, 17:55
20m
Lobby and Hallway , 2nd Floor

Lobby and Hallway , 2nd Floor

Poster Reference Materials, Carriers, Intercomparisons Poster Session B

Speaker

David Lund (University of Notre Dame)

Description

The isotope $^{129}$I, with a half-life of 15.7 million years, serves critical roles ranging from an environmental tracer of fission products to a significant marker in nuclear astrophysics. Due to its low natural terrestrial abundance (approximately one part per trillion), accelerator mass spectrometry (AMS) offers a robust method for its detection, accurately distinguishing the $^{129}$I signal from the stable isotope $^{127}$I in aqueous samples. Recent advancements in our beamline configuration and time-of-flight detection systems at the University of Notre Dame’s Nuclear Science Laboratory have significantly increased our measurement sensitivity for $^{129}$I. This study presents a comprehensive analysis of reference standards, highlighting the enhanced detection capabilities achieved. The modifications to the AMS system, improved time-of-flight resolution, detailed analysis results, and implications for environmental and astrophysical applications will be discussed. In particular, we will highlight our collaboration with the nuclear theory group at Notre Dame, and how future experiments may be used to build upon advancements made by Wang et al. (2021, 2023) on the understanding of certain astrophysical processes (Wang, X., Clark, A. M., Ellis, J., et al. 2021, r-Process Radioisotopes from Near-Earth Supernovae and Kilonovae), (Wang, X., Clark, A. M., Ellis, J., et al. 2023, Proposed Lunar Measurements of r-process Radioisotopes to Distinguish the Origin of Deep-sea $^{244}$Pu).

This work is supported by the National Science Foundation Grant No. NSF PHY-2011890.

Student Submission Yes

Primary authors

David Lund (University of Notre Dame) Calvin Bacall (University of Notre Dame) Thomas Bailey (University of Notre Dame) Prof. Philippe Collon (University of Notre Dame) Griffin Mulcahy (University of Notre Dame) Will Peeler (University of Notre Dame)

Presentation materials

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